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Takai, Shizuka; Shimada, Taro; Takeda, Seiji; Koike, Katsuaki*
Mathematical Geosciences, 56(2), p.333 - 360, 2024/02
Times Cited Count：0 Percentile：0.01(Geosciences, Multidisciplinary)To enable proper remediation of accidental groundwater contamination, the contaminant plume evolution needs to be accurately estimated. In the estimation, uncertainties in both the contaminant source and hydrogeological structure should be considered, especially the temporal release history and hydraulic transmissivity. Although the release history can be estimated using geostatistical approaches, previous studies use the deterministic hydraulic property field. Geostatistical approaches can also effectively estimate an unknown heterogeneous transmissivity field via the joint data use, such as a combination of hydraulic head and tracer data. However, tracer tests implemented over a contaminated area necessarily disturb the in situ condition of the contamination. Conversely, measurements of the transient concentration data over an area are possible and can preserve the conditions. Accordingly, this study develops a geostatistical method for the joint clarification of contaminant plume and transmissivity distributions using both head and contaminant concentration data. The applicability and effectiveness of the proposed method are demonstrated through two numerical experiments assuming a two-dimensional heterogenous confined aquifer. The use of contaminant concentration data is key to accurate estimation of the transmissivity. The accuracy of the proposed method using both head and concentration data was verified achieving a high linear correlation coefficient of 0.97 between the true and estimated concentrations for both experiments, which was 0.67 or more than the results using only the head data. Furthermore, the uncertainty of the contaminant plume evolution was successfully evaluated by considering the uncertainties of both the initial plume and the transmissivity distributions, based on their conditional realizations.
Pt-labeled platinum complex and evaluation of its biodistribution in healthy miceOmokawa, Marina*; Kimura, Hiroyuki*; Hatsukawa, Yuichi*; Kawashima, Hidekazu*; Tsukada, Kazuaki; Yagi, Yusuke*; Naito, Yuki*; Yasui, Hiroyuki*
Bioorganic & Medicinal Chemistry, 97, p.117557_1 - 117557_6, 2024/01
Times Cited Count：0 Percentile：0.01(Biochemistry & Molecular Biology)Tanaka, Masaaki; Miyake, Yasuhiro*; Ezure, Toshiki; Hamase, Erina
Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 9 Pages, 2023/05
The numerical analysis model for the computational fluid dynamics (CFD) code for the design study is developed to evaluate the thermal-hydraulics in the core under the core-plenum interaction (CPI) during the decay heat removal using the dipped type direct heat exchanger (D-DHX). To judge the adequacy of the numerical results for a validation study with the sodium experiment results conducted at PLANDTL-2 facility, the degree of difference (DoD) between the numerical and experimental results must be measured by using the area validation metrics (AVM). Through the examinations, the applicability of the AVM and MAVM based on the p-box method was confirmed.
Ueki, Taro
Progress in Nuclear Energy, 159, p.104630_1 - 104630_9, 2023/05
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)In this work, the methodology of Generalized Extreme Value (GEV) is applied to criticality tallies in Monte Carlo fission source cycles in order to evaluate the utility value of the distribution tail ends. Numerical results obtained under a sufficiently large number of particles per cycle show that the extreme value index (EVI) in GEV falls within the range of Weibull distribution including the EVI of Gumbel distribution as the role of a boundary value layer. GEV is also applied to a historically-challenging loosely-coupled system for demonstrating population diagnosis under an insufficient number of particles per cycle. It turns out that the transition from one equilibrium to other equilibrium makes the EVIs of upper and lower distribution tail ends depart from each other so that one of them falls in the range of Weibull distribution and the other in that of Frechet distribution.
Kawahara, Rika*; Ochi, Kotaro; Yamaguchi, Katsuhiko*; Torii, Tatsuo*
Hoshasen (Internet), 48(2), p.43 - 48, 2023/04
The accident at the Fukushima Daiichi NPP resulted in a large amount of radioactive material being dispersed into the surrounding environment. It is important to understand the radiation distribution in the area, which is still located in the difficult-to-return zone. In this study, a Compton camera and an optical camera were combined to produce a three-dimensional distribution map of source locations and their intensities. Two locations in the difficult-to-return zone (Okuma town) were surveyed: a park parking lot and the area around a private house. The distribution of air dose rates was determined by measurements with a survey meter with a wand-type GPS (Gamma Plotter H manufactured by Nippon Radiation Engineering Co. Measurements were taken with a Compton camera (H420, H3D, USA) at several different positions and angles towards the hotspots. The software (Application Programming Interface Example) allowed real-time confirmation of the radiation incident information (incident time, energy, x, y, z) obtained by the Compton camera. By photographing hotspots in high-dose areas from different positions and angles, the location of the radiation sources and their spatial extent could be confirmed.
Takai, Shizuka; Shimada, Taro; Takeda, Seiji; Koike, Katsuaki*
Journal of Contaminant Hydrology, 251, p.104097_1 - 104097_12, 2022/12
Times Cited Count：3 Percentile：49.4(Environmental Sciences)When assessing the risk from an underground environment that is contaminated by radioactive nuclides and hazardous chemicals and planning for remediation, the contaminant plume distribution and the associated uncertainty from measured data should be estimated accurately. While the release history of the contaminant plume may be unknown, the extent of the plume caused by a known source and the associated uncertainty can be calculated inversely from the concentration data using a geostatistical method that accounts for the temporal correlation of its release history and groundwater flow modeling. However, the preceding geostatistical approaches have three drawbacks: (1) no applications of the three-dimensional plume estimation in real situations, (2) no constraints for the estimation of the plume distribution, which can yield negative concentration and large uncertainties, and (3) few applications to actual cases with multiple contaminants. To address these problems, the non-negativity constraint using Gibbs sampling was incorporated into the geostatistical method with groundwater flow modeling for contaminant plume estimation. This method was then tested on groundwater contamination in the Gloucester landfill in Ontario, Canada. The method was applied to three water soluble organic contaminants: 1,4-dioxane, tetrahydrofuran, and diethyl ether. The effectiveness of the proposed method was verified by the general agreement of the calculated plume distributions of the three contaminants with concentration data from 66 points in 1982 (linear correlation coefficient of about 0.7). In particular, the reproduced large spill of organic contaminants of 1,4-dioxane in 1978 was more accurate than the result of preceding minimum relative entropy-based studies. The same peak also appeared in the tetrahydrofuran and diethyl ether distributions approximately within the range of the retardation factor derived from the fraction of organic carbon.
Suzuki, Gen*; Ishikawa, Tetsuo*; Oba, Takashi*; Hasegawa, Arifumi*; Nagai, Haruyasu; Miyatake, Hirokazu*; Yoshizawa, Nobuaki*
Journal of Radiation Research (Internet), 63(6), p.796 - 804, 2022/11
Times Cited Count：2 Percentile：27.14(Biology)To elucidate the association between radiation dose and thyroid cancer after the 2011 Fukushima Daiichi Nuclear Power Station (FDNPS) accident, it is essential to estimate individual thyroid equivalent doses (TEDs) to children. In a previous study, we reported a methodology for reconstructing TEDs from inhalation based on individual behavioural survey sheets combined with a spatiotemporal radionuclides database constructed by an atmospheric transport, diffusion, and deposition model (ATDM). In the present study, we further refined our methodology and estimated the combined TEDs from inhalation and ingestion among children in 16 municipalities around the nuclear power station utilizing 3,256 individual whereabouts questionnaire survey sheets. Distributions of estimated TEDs were similar to estimates based on direct thyroid measurements in 1080 children in Iwaki City, Kawamata Town, Iitate Village, and Minamisoma City. Mean TEDs in 1-year-old children ranged from 1.3 mSv in Date City to 14.9 mSv in Odaka Ward in Minamisoma City, and the 95th percentiles varied from 2.3 mSv in Date City to 28.8 mSv in Namie Town. In the future, this methodology can be useful for a case-control study of thyroid cancer after the FDNPS accident.
Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*
Hoshasen (Internet), 47(3), p.89 - 96, 2022/10
Torii, Tatsuo; Sanada, Yukihisa
Keisoku Gijutsu, 50(11), p.23 - 28, 2022/10
no abstracts in English
Sakaki, Koji*; Kim, H.*; Majzoub, E. H.*; Machida, Akihiko*; Watanuki, Tetsu*; Ikeda, Kazutaka*; Otomo, Toshiya*; Mizuno, Masataka*; Matsumura, Daiju; Nakamura, Yumiko*
Acta Materialia, 234, p.118055_1 - 118055_10, 2022/08
Times Cited Count：9 Percentile：83.6(Materials Science, Multidisciplinary)Takai, Shizuka; Namekawa, Masakazu*; Shimada, Taro; Takeda, Seiji
IEEE Transactions on Nuclear Science, 69(7), p.1789 - 1798, 2022/07
Times Cited Count：0 Percentile：0.01(Engineering, Electrical & Electronic)To reduce a large amount of contaminated concrete rubble stored in the Fukushima Daiichi Nuclear Power Station site, recycling low-radioactivity rubble within the site is a possible remedy. To promote recycling while ensuring safety, not only the average radioactivity but also the radioactivity distribution of concrete rubble should be efficiently evaluated because the details of rubble contamination caused by the accident remain unclear and likely include hotspots. However, evaluating inhomogeneous contamination of thick and/or dense materials is difficult using previous measurement systems, such as clearance monitors. This study experimentally confirmed the potential applicability of image reconstruction algorithms for radioactivity distribution evaluation in concrete rubble filled in a chamber. Radiation was measured using plastic scintillation fiber around the chamber (50 
50 40 cm
). Localized hotspots were simulated using standard sources of 
Cs, which is one of the main nuclides of contaminated rubble. The radioactivity distribution was calculated for 100 or 50 voxels (voxel size: (10 cm) or 10 10 20 cm) constituting the chamber. For 100 voxels, inner hotspots were undetected, whereas, for 50 voxels, both inner and surface hotspots were reconstructible. The distribution evaluated using the maximum likelihood expectation maximization algorithm was the most accurate; the average radioactivity was estimated within 70% accuracy in all seven cases.
Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*
Nuclear Instruments and Methods in Physics Research A, 1034, p.166793_1 - 166793_6, 2022/07
Times Cited Count：2 Percentile：53.91(Instruments & Instrumentation)
rays from the 
-wave resonance of 
SnKoga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.
Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05
Times Cited Count：3 Percentile：66.85(Physics, Nuclear)no abstracts in English
Ochi, Kotaro; Funaki, Hironori; Yoshimura, Kazuya; Iimoto, Takeshi*; Matsuda, Norihiro; Sanada, Yukihisa
Radiation and Environmental Biophysics, 61(1), p.147 - 159, 2022/03
Times Cited Count：2 Percentile：47.19(Biology)Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*; Yamazaki, Atsushi*; Sato, Yuki; Torii, Tatsuo; Wakaida, Ikuo
Journal of Nuclear Engineering and Radiation Science, 7(4), p.042002_1 - 042002_7, 2021/10
For the application in the measurement of the high dose rate hot spots inside the Fukushima Daiichi Nuclear Power Station (FDNPS) buildings, we propose a novel one-dimensional radiation distribution sensing method using an optical fiber sensor based on wavelength spectrum unfolding. The proposed method estimates the incident position of radiation to the fiber by the unfolding of the wavelength spectrum output from the fiber edge using the fact that the attenuation length of light along the fiber depends on the wavelength. Because this method measures the integrated light intensity, this method can avoid the problem of counting loss and signal pile-up, which occurs in the radiation detector with pulse counting mode under high dose rate field. Through basic experiments using the ultraviolet light source and 
Sr/Y radioactive point source, basic properties of source position detection were confirmed.
random mediaAraki, Shohei; Yamane, Yuichi; Ueki, Taro; Tonoike, Kotaro
Nuclear Science and Engineering, 195(10), p.1107 - 1117, 2021/10
Times Cited Count：2 Percentile：31.78(Nuclear Science & Technology)Criticality control of random media such as fuel debris is one of the most important safety issues in post-accident management. 
spectrum randomizing model is expected to simulate such random media because it is well known that the noise can describe a diverse range of random and disordered natural phenomena. In this paper, we focused on the relationship between the multiplication factor and moderation condition in the random media. A number of random media were realized with the spectrum randomizing model that is based on the Randomized Weierstrass function (RWF). The volume ratio of concrete to fuel was adopted as an index for the moderation condition. The multiplication factors were calculated with a two-energy group Monte Carlo calculation. The calculation results were analyzed by using variance, skewness, and kurtosis. Those statistical parameters had an extreme value around the optimum moderation condition. This result suggested that it is possible to predict the rough trend of variation range, distortion, and outlier of multiplication factors in the random media.
Kim, M.; Malins, A.; Machida, Masahiko; Yoshimura, Kazuya; Saito, Kimiaki; Yoshida, Hiroko*; Yanagi, Hideaki*; Yoshida, Toru*; Hasegawa, Yukihiro*
RIST News, (67), p.3 - 15, 2021/09
no abstracts in English
Uchida, Shunsuke; Karasawa, Hidetoshi; Kino, Chiaki*; Pellegrini, M.*; Naito, Masanori*; Osaka, Masahiko
Nuclear Engineering and Design, 380, p.111256_1 - 111256_19, 2021/08
Times Cited Count：6 Percentile：72.21(Nuclear Science & Technology)It is essential to grasp the long-term distributions of FP as well as fuel debris all over the Fukushima Daiichi Nuclear Power Plant (1F) for safe completion of its decommissioning projects. The fuel debris is going to be removed from the plant under the severe conditions of FP being scattered during major decommissioning work, and then, the decommissioning projects are going to be terminated by storing safely the removed debris as recovered fertile materials or as materials for final radioactive disposal. In order to determine the FP distribution in the plant for the long period from the accident occurrence to the termination of the plant decommissioning, procedures for analyzing multi-term FP behaviors were proposed. The proposed procedures should be improved by applying the FP data measured in the plant and validated based on the feedback data. Then, the accuracy-improved procedures should be applied to estimate FP distribution during each period of the decommissioning projects.
Uchida, Shunsuke; Pellegrini, M.*; Naito, Masanori*
Nuclear Engineering and Design, 380, p.111303_1 - 111303_11, 2021/08
Times Cited Count：1 Percentile：16.35(Nuclear Science & Technology)Multi-term FP analysis procedures were developed to determine FP distribution all over F1 not only for analyzing accident propagation but also for planning its decommissioning projects. They should be validated based on the measured FP data. One of the useful tools for their validation was application of the dose rate data monitored by the containment atmosphere monitoring system (CAMS). However, in order to compare the data with different characteristics and dimensional units, e.g., FP distribution (kg, Bq) and dose rate (Sv/h), application of the conversion factors bridging them would be effective and useful. In order to prepare speedy, easy-to-handle and tractable procedures to calculate radiation dose rates at the CAMS detector locations, dose rate conversion factors were determined for major source locations and major radionuclides. The dose rates could be easily calculated by multiplying FP amounts obtained with the multiterm FP analysis procedures by the conversion factors.
Hirouchi, Jun; Takahara, Shogo; Yoshimura, Kazuya
Journal of Environmental Radioactivity, 232, p.106572_1 - 106572_6, 2021/06
Times Cited Count：1 Percentile：6.09(Environmental Sciences)Information on the radioactivity distribution inside and outside houses is useful for indoor external dose assessments. In this study, we collected both soil samples around the target houses and house material samples (i.e., of the floor, inner wall, ceiling, outer wall, and roof). The radioactivity of the samples was measured using a high-purity germanium detector. The surface contamination densities of the floor, inner wall, ceiling, outer wall, and roof relative to the ground were 3 10
7 10
, 6 10
4 10
, 7 103 10, 2 101 10, and 4 102 10
, respectively. The relative surface contamination densities varied depending on the material, its location, and the orientation of the surface.
